Take a look at the section on volunteering with prisoners and ex-offenders and you will find some great opportunities for working within the prison service, helping prisoners to rehabilitate themselves as well as offering a friendly ear and advice.

You could also try PACT (Prison Advice and Care Trust). They list opportunities on offer in the different areas of the prison service. 

The HM Prison Service has an entire section listing organisations they work with and who offer support to prisoners.

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